Hyperfine interaction in a quantum dot: Non-Markovian electron spin dynamics

We have performed a systematic calculation for the non-Markovian dynamics of a localized electron spin interacting with an environment of nuclear spins via the Fermi contact hyperfine interaction. This work applies to an electron in the s -type orbital ground state of a quantum dot or bound to a donor impurity, and is valid for arbitrary polarization p of the nuclear spin system, and arbitrary nuclear spin I in high magnetic fields. In the limit of p=1 and I=1/2, the Born approximation of our perturbative theory recovers the exact electron spin dynamics. We have found the form of the generalized master equation (GME) for the longitudinal and transverse components of the electron spin to all orders in the electron spin--nuclear spin flip-flop terms. Our perturbative expansion is regular, unlike standard time-dependent perturbation theory, and can be carried-out to higher orders. We show this explicitly with a fourth-order calculation of the longitudinal spin dynamics. In zero magnetic field, the fraction of the electron spin that decays is bounded by the smallness parameter \delta=1/p^{2}N, where N is the number of nuclear spins within the extent of the electron wave function. However, the form of the decay can only be determined in a high magnetic field, much larger than the maximum Overhauser field. In general the electron spin shows rich dynamics, described by a sum of contributions with non-exponential decay, exponential decay, and undamped oscillations. There is an abrupt crossover in the electron spin asymptotics at a critical dimensionality and shape of the electron envelope wave function. We propose a scheme that could be used to measure the non-Markovian dynamics using a standard spin-echo technique, even when the fraction that undergoes non-Markovian dynamics is small.Comment: 22 pages, 8 figure

Spin-dependent Andreev reflection tunneling through a quantum dot with intradot spin-flip scattering

We study Andreev reflection (AR) tunneling through a quantum dot (QD) connected to a ferromagnet and a superconductor, in which the intradot spin-flip interaction is included. By using the nonequibrium-Green-function method, the formula of the linear AR conductance is derived at zero temperature. It is found that competition between the intradot spin-flip scattering and the tunneling coupling to the leads dominantes resonant behaviours of the AR conductance versus the gate voltage.A weak spin-flip scattering leads to a single peak resonance.However, with the spin-flip scattering strength increasing, the AR conductance will develop into a double peak resonannce implying a novel structure in the tunneling spectrum of the AR conductance. Besides, the effect of the spin-dependent tunneling couplings, the matching of Fermi velocity, and the spin polarization of the ferromagnet on the AR conductance is eximined in detail.Comment: 14 pages, 4 figure

Comment on "Spin relaxation in quantum Hall systems"

W. Apel and Yu.A. Bychkov have recently considered the spin relaxation in a 2D quantum Hall system for the filling factor close to unity [PRL v.82, 3324 (1999)]. The authors considered only one spin flip mechanism (direct spin-phonon coupling) among several possible spin-orbit related ones and came to the conclusion that the spin relaxation time due to this mechanism is quite short: around $10^{-10}$ s at B=10 T (for GaAs). This time is much shorter than the typical time ($10^{-5}$ s) obtained earlier by D. Frenkel while considering the spin relaxation of 2D electrons in a quantizing magnetic field without the Coulomb interaction and for the same spin-phonon coupling. I show that the authors' conclusion about the value of the spin-flip time is wrong and have deduced the correct time which is by several orders of magnitude longer. I also discuss the admixture mechanism of the spin-orbit interaction.Comment: 1 pag

Electron spin evolution induced by interaction with nuclei in a quantum dot

We study the decoherence of a single electron spin in an isolated quantum dot induced by hyperfine interaction with nuclei for times smaller than the nuclear spin relaxation time. The decay is caused by the spatial variation of the electron envelope wave function within the dot, leading to a non-uniform hyperfine coupling $A$. We show that the usual treatment of the problem based on the Markovian approximation is impossible because the correlation time for the nuclear magnetic field seen by the electron spin is itself determined by the flip-flop processes. The decay of the electron spin correlation function is not exponential but rather power (inverse logarithm) law-like. For polarized nuclei we find an exact solution and show that the precession amplitude and the decay behavior can be tuned by the magnetic field. The decay time is given by $\hbar N/A$, where $N$ is the number of nuclei inside the dot. The amplitude of precession, reached as a result of the decay, is finite. We show that there is a striking difference between the decoherence time for a single dot and the dephasing time for an ensemble of dots.Comment: Revtex, 11 pages, 5 figure

Effect of external magnetic field on electron spin dephasing induced by hyperfine interaction in quantum dots

We investigate the influence of an external magnetic field on spin phase relaxation of single electrons in semiconductor quantum dots induced by the hyperfine interaction. The basic decay mechanism is attributed to the dispersion of local effective nuclear fields over the ensemble of quantum dots. The characteristics of electron spin dephasing is analyzed by taking an average over the nuclear spin distribution. We find that the dephasing rate can be estimated as a spin precession frequency caused primarily by the mean value of the local nuclear magnetic field. Furthermore, it is shown that the hyperfine interaction does not fully depolarize electron spin. The loss of initial spin polarization during the dephasing process depends strongly on the external magnetic field, leading to the possibility of effective suppression of this mechanism.Comment: 10 pages, 2 figure

Spin decay and quantum parallelism

We study the time evolution of a single spin coupled inhomogeneously to a spin environment. Such a system is realized by a single electron spin bound in a semiconductor nanostructure and interacting with surrounding nuclear spins. We find striking dependencies on the type of the initial state of the nuclear spin system. Simple product states show a profoundly different behavior than randomly correlated states whose time evolution provides an illustrative example of quantum parallelism and entanglement in a decoherence phenomenon.Comment: 6 pages, 4 figures included, version to appear in Phys. Rev.

Hyperfine-mediated transitions between a Zeeman split doublet in GaAs quantum dots: The role of the internal field

We consider the hyperfine-mediated transition rate between Zeeman split spin states of the lowest orbital level in a GaAs quantum dot. We separate the hyperfine Hamiltonian into a part which is diagonal in the orbital states and another one which mixes different orbitals. The diagonal part gives rise to an effective (internal) magnetic field which, in addition to an external magnetic field, determines the Zeeman splitting. Spin-flip transitions in the dots are induced by the orbital mixing part accompanied by an emission of a phonon. We evaluate the rate for different regimes of applied magnetic field and temperature. The rates we find are bigger that the spin-orbit related rates provided the external magnetic field is sufficiently low.Comment: 8 pages, 3 figure

Hole spin relaxation in semiconductor quantum dots

Hole spin relaxation time due to the hole-acoustic phonon scattering in GaAs quantum dots confined in quantum wells along (001) and (111) directions is studied after the exact diagonalization of Luttinger Hamiltonian. Different effects such as strain, magnetic field, quantum dot diameter, quantum well width and the temperature on the spin relaxation time are investigated thoroughly. Many features which are quite different from the electron spin relaxation in quantum dots and quantum wells are presented with the underlying physics elaborated.Comment: 10 pages, 10 figure

Spin relaxation at the singlet-triplet crossing in a quantum dot

We study spin relaxation in a two-electron quantum dot in the vicinity of the singlet-triplet crossing. The spin relaxation occurs due to a combined effect of the spin-orbit, Zeeman, and electron-phonon interactions. The singlet-triplet relaxation rates exhibit strong variations as a function of the singlet-triplet splitting. We show that the Coulomb interaction between the electrons has two competing effects on the singlet-triplet spin relaxation. One effect is to enhance the relative strength of spin-orbit coupling in the quantum dot, resulting in larger spin-orbit splittings and thus in a stronger coupling of spin to charge. The other effect is to make the charge density profiles of the singlet and triplet look similar to each other, thus diminishing the ability of charge environments to discriminate between singlet and triplet states. We thus find essentially different channels of singlet-triplet relaxation for the case of strong and weak Coulomb interaction. Finally, for the linear in momentum Dresselhaus and Rashba spin-orbit interactions, we calculate the singlet-triplet relaxation rates to leading order in the spin-orbit interaction, and find that they are proportional to the second power of the Zeeman energy, in agreement with recent experiments on triplet-to-singlet relaxation in quantum dots.Comment: 29 pages, 14 figures, 1 tabl